My research is essentially based on the internal
dynamics of volatile elements (C, N, H, S) and to elucidate the processes that
control their long-term distribution in the different terrestrial reservoirs
(oceans, oceanic and continental crust, upper and lower mantle). Their study
provides a better understanding of their initial state, i.e. 4.5 billion years
ago, and thus understand the origin and chronology of their contribution, for
example understanding what type of meteorites contributed to the presence of
water on Earth and when they were brought in (after or before the impact that
generated the Moon?).
During the first fifteen years of my career, with my
colleagues and students, we concentrated on the study of the nitrogen cycle -
in particular through the study of diamonds for which nitrogen is the major
impurity, with in parallel several works on rocks in subduction zones, mid
ocean-ridge basalts and hot spots. Amongst other results, we highlighted the
'massive recycling' of nitrogen in the mantle and have shown that, contrary to
popular belief, that most so-called 'ecologic' diamonds are not formed from
surface carbon recycling.
Since 2008, after having set up methods for analysing the three isotope ratios of sulphur,
I extended my investigations to the sulphur cycle.
Among our main results, we were able to demonstrate that sulphur
isotopes are very good tracers of chemical geodynamics (i.e. recycling of
surface material) and that the mantle retains the signature of sulphur sequestration in the earth's core. Our current work
is interested in better establishing the fate and flux of sulphur
recycled in the mantle.
My research, using the three isotopic ratios of sulphur and oxygen, falls more generally speaking on the frame
of better understanding and applying 'mass-independent isotope fractionation'
(MIF), with several recent works in the field of atmospheric chemistry,
focusing on the formation of sulphate aerosols, where we provided some original
constraints on their formation. Our on-going work concerns more fundamental
aspects of mechanisms for generating MIF, particularly during evaporation
processes and heterogeneous gas/solid chemical reactions.
In parallel, through several collaborations, I am
collaborating with several cool colleagues on the study of ancient
paleo-environmental conditions (> 2.3 billion years, ~ 630 million years, 8
million years) for which sulphur isotopes allow us to
deduce e.g. the presence/absence/appearance of atmospheric oxygen, and the
types of organisms present.